我会考虑哪些最适合您的需求和客户需求以及将使用该应用程序的人员所支持的技术。 

I would look at what best suits your needs and customer needs along with what technology is supported for those who will use the application. 

使用Android的想法请参阅从Windows C＃App操纵Android设备。

For an idea on working with Android see Manipulating Android Devices from a Windows C# App.

另外，Microsoft表示Windows表格将受到很长时间的支持，但.NET Core库会支持Windows表单。

On a side note, Windows forms will be supported for a long time by Microsoft but more so with .NET Core libraries.